The invention discloses a 
macro preparation device and method of carboxyl 
functionalized graphene and belongs to the technical field of preparation of 
graphene. The 
macro preparation device comprisesa first dispersion kettle, an activation reactor, a first filtering and washing 
tower, a second dispersion kettle, a reaction kettle, a second filtering and washing 
tower, a third dispersion kettle, adrying 
tower, a first 
storage tank and a second 
storage tank, wherein the first dispersion kettle, the activation reactor, the first filtering and washing tower, the second dispersion kettle, the reaction kettle, the second filtering and washing tower, the third dispersion kettle and the 
drying tower are connected in sequence; the first filtering and washing tower, the first 
storage tank and thefirst dispersion kettle are connected in sequence; the second filtering and washing tower, the second storage tank and the second dispersion kettle are connected in sequence. The 
macro preparation device and method of the carboxyl 
functionalized graphene, disclosed by the invention, have the advantages of simple and compact structure, reasonable design, high continuous degree and less equipment investment; the carboxyl 
functionalized graphene can be efficiently prepared and the production cost is reduced.